Co-reporter:Ilya Belopolski;Su-Yang Xu;Nikesh Koirala;Chang Liu;Guang Bian;Vladimir N. Strocov;Guoqing Chang;Madhab Neupane;Nasser Alidoust;Daniel Sanchez;Hao Zheng;Matthew Brahlek;Victor Rogalev;Timur Kim;Nicholas C. Plumb;Chaoyu Chen;François Bertran;Patrick Le Fèvre;Amina Taleb-Ibrahimi;Maria-Carmen Asensio;Ming Shi;Hsin Lin;Moritz Hoesch;Seongshik Oh
Science Advances 2017 Vol 3( Iss 3) pp:
Publication Date(Web):24 Mar 2017
DOI: 10.1126/sciadv.1501692
Topologically protected electron states arranged artificially in real space form a highly tunable emergent atomic chain.
Co-reporter:Guoqing Chang;Su-Yang Xu;Daniel S. Sanchez;Shin-Ming Huang;Chi-Cheng Lee;Tay-Rong Chang;Guang Bian;Nasser Alidoust;Ilya Belopolski;Arun Bansil;Hsin Lin;Horng-Tay Jeng;Hao Zheng
Science Advances 2016 Volume 2(Issue 6) pp:
Publication Date(Web):
DOI:10.1126/sciadv.1600295
A new methodology is used to design robust Weyl semimetals and to identify the most robust and ideal Weyl semimetal candidate in Ta3S2.
Co-reporter:Hao Zheng, Su-Yang Xu, Guang Bian, Cheng Guo, Guoqing Chang, Daniel S. Sanchez, Ilya Belopolski, Chi-Cheng Lee, Shin-Ming Huang, Xiao Zhang, Raman Sankar, Nasser Alidoust, Tay-Rong Chang, Fan Wu, Titus Neupert, Fangcheng Chou, Horng-Tay Jeng, Nan Yao, Arun Bansil, Shuang Jia, Hsin Lin, and M. Zahid Hasan
ACS Nano 2016 Volume 10(Issue 1) pp:1378
Publication Date(Web):January 8, 2016
DOI:10.1021/acsnano.5b06807
Weyl semimetals may open a new era in condensed matter physics, materials science, and nanotechnology after graphene and topological insulators. We report the first atomic scale view of the surface states of a Weyl semimetal (NbP) using scanning tunneling microscopy/spectroscopy. We observe coherent quantum interference patterns that arise from the scattering of quasiparticles near point defects on the surface. The measurements reveal the surface electronic structure both below and above the chemical potential in both real and reciprocal spaces. Moreover, the interference maps uncover the scattering processes of NbP’s exotic surface states. Through comparison between experimental data and theoretical calculations, we further discover that the orbital and/or spin texture of the surface bands may suppress certain scattering channels on NbP. These results provide a comprehensive understanding of electronic properties on Weyl semimetal surfaces.Keywords: scanning tunneling microscopy; topological matter; Weyl semimetal;
Co-reporter:Guang Bian, Zhengfei Wang, Xiao-Xiong Wang, Caizhi Xu, SuYang Xu, Thomas Miller, M. Zahid Hasan, Feng Liu, and Tai-Chang Chiang
ACS Nano 2016 Volume 10(Issue 3) pp:3859
Publication Date(Web):March 1, 2016
DOI:10.1021/acsnano.6b00987
We report on the fabrication of a two-dimensional topological insulator Bi(111) bilayer on Sb nanofilms via a sequential molecular beam epitaxy growth technique. Our angle-resolved photoemission measurements demonstrate the evolution of the electronic band structure of the heterostructure as a function of the film thickness and reveal the existence of a two-dimensional spinful massless electron gas within the top Bi bilayer. Interestingly, our first-principles calculation extrapolating the observed band structure shows that, by tuning down the thickness of the supporting Sb films into the quantum dimension regime, a pair of isolated topological edge states emerges in a partial energy gap at 0.32 eV above the Fermi level as a consequence of quantum confinement effect. Our results and methodology of fabricating nanoscale heterostructures establish the Bi bilayer/Sb heterostructure as a platform of great potential for both ultra-low-energy-cost electronics and surface-based spintronics.Keywords: Bi(111) bilayer; Kane−Mele model; quantum spin Hall effect; quantum well states
Co-reporter:Shin-Ming Huang;Su-Yang Xu;Guoqing Chang;Guang Bian;Ilya Belopolski;Chi-Cheng Lee;Nasser Alidoust;Horng-Tay Jeng;BaoKai Wang;Madhab Neupane;Tay-Rong Chang;Daniel Sanchez;Hao Zheng;Arun Bansil;Titus Neupert;Hsin Lin
PNAS 2016 Volume 113 (Issue 5 ) pp:1180-1185
Publication Date(Web):2016-02-02
DOI:10.1073/pnas.1514581113
Weyl semimetals have attracted worldwide attention due to their wide range of exotic properties predicted in theories. The
experimental realization had remained elusive for a long time despite much effort. Very recently, the first Weyl semimetal
has been discovered in an inversion-breaking, stoichiometric solid TaAs. So far, the TaAs class remains the only Weyl semimetal
available in real materials. To facilitate the transition of Weyl semimetals from the realm of purely theoretical interest
to the realm of experimental studies and device applications, it is of crucial importance to identify other robust candidates
that are experimentally feasible to be realized. In this paper, we propose such a Weyl semimetal candidate in an inversion-breaking,
stoichiometric compound strontium silicide, SrSi2, with many new and novel properties that are distinct from TaAs. We show that SrSi2 is a Weyl semimetal even without spin–orbit coupling and that, after the inclusion of spin–orbit coupling, two Weyl fermions
stick together forming an exotic double Weyl fermion with quadratic dispersions and a higher chiral charge of ±2. Moreover,
we find that the Weyl nodes with opposite charges are located at different energies due to the absence of mirror symmetry
in SrSi2, paving the way for the realization of the chiral magnetic effect. Our systematic results not only identify a much-needed
robust Weyl semimetal candidate but also open the door to new topological Weyl physics that is not possible in TaAs.
Co-reporter:Su-Yang Xu;Nasser Alidoust;Ilya Belopolski;Raman Sankar;Guoqing Chang;Madhab Neupane;Daniel S. Sanchez;Chenglong Zhang;Shin-Ming Huang;Guang Bian;Zhujun Yuan;Chi-Cheng Lee;BaoKai Wang;Jie Ma;Hao Zheng;Arun Bansil;Fangcheng Chou;Pavel P. Shibayev;Hsin Lin;Shuang Jia
Science 2015 Volume 349(Issue 6248) pp:613-617
Publication Date(Web):07 Aug 2015
DOI:10.1126/science.aaa9297
Weyl physics emerges in the laboratory
Weyl fermions—massless particles with half-integer spin—were once mistakenly thought to describe neutrinos. Although not yet observed among elementary particles, Weyl fermions may exist as collective excitations in so-called Weyl semimetals. These materials have an unusual band structure in which the linearly dispersing valence and conduction bands meet at discrete “Weyl points.” Xu et al. used photoemission spectroscopy to identify TaAs as a Weyl semimetal capable of hosting Weyl fermions. In a complementary study, Lu et al. detected the characteristic Weyl points in a photonic crystal. The observation of Weyl physics may enable the discovery of exotic fundamental phenomena.
Science, this issue p. 613 and 622
Co-reporter:Ilya Belopolski;Su-Yang Xu;Daniel S. Sanchez;Chenglong Zhang;Guoqing Chang;Cheng Guo;Guang Bian;Zhujun Yuan;Hong Lu;Tay-Rong Chang;Pavel P. Shibayev;Mykhailo L. Prokopovych;Nasser Alidoust;Hao Zheng;Chi-Cheng Lee;Shin-Ming Huang;Raman Sankar;Fangcheng Chou;Chuang-Han Hsu;Horng-Tay Jeng;Arun Bansil;Titus Neupert;Vladimir N. Strocov;Hsin Lin;Shuang Jia
Science Advances 2015 Volume 1(Issue 10) pp:
Publication Date(Web):
DOI:10.1126/sciadv.1501092
Photoemission established tantalum phosphide as a Weyl semimetal, which hosts exotic Weyl fermion quasiparticles and Fermi arcs.
Co-reporter:Chang Liu;Su-Yang Xu;Satya K. Kushwaha;Raman Sankar;Jason W. Krizan;Ilya Belopolski;Madhab Neupane;Guang Bian;Nasser Alidoust;Tay-Rong Chang;Horng-Tay Jeng;Cheng-Yi Huang;Wei-Feng Tsai;Hsin Lin;Pavel P. Shibayev;Fang-Cheng Chou;Robert J. Cava
Science 2015 Volume 347(Issue 6219) pp:294-298
Publication Date(Web):16 Jan 2015
DOI:10.1126/science.1256742
Nailing down the topology of a semimetal
Topological insulators are exotic materials that have a conducting surface state that can withstand certain types of material imperfection. Theoreticians have predicted a different kind of surface state in related three-dimensional topological Dirac semimetals, which do not have an energy gap in the band structure of the bulk. Xu et al. used photoemission spectroscopy to map out the band structure of the material Na3Bi and detected the predicted surface state. Their results may lead to further insights into the physics of topological matter.
Science, this issue p. 294
Co-reporter:Su-Yang Xu;Y. Xia;L. A. Wray;S. Jia;F. Meier;J. H. Dil;J. Osterwalder;B. Slomski;A. Bansil;H. Lin;R. J. Cava;M. Z. Hasan
Science 2011 Volume 332(Issue 6029) pp:560-564
Publication Date(Web):29 Apr 2011
DOI:10.1126/science.1201607
Two types of bulk insulator are realized in the same family of compounds through chemical doping.
Co-reporter:D. Hsieh;Y. Xia;L. Wray;D. Qian;A. Pal;J. H. Dil;J. Osterwalder;F. Meier;G. Bihlmayer;C. L. Kane;Y. S. Hor;R. J. Cava;M. Z. Hasan
Science 2009 Vol 323(5916) pp:919-922
Publication Date(Web):13 Feb 2009
DOI:10.1126/science.1167733
Abstract
A topologically ordered material is characterized by a rare quantum organization of electrons that evades the conventional spontaneously broken symmetry–based classification of condensed matter. Exotic spin-transport phenomena, such as the dissipationless quantum spin Hall effect, have been speculated to originate from a topological order whose identification requires a spin-sensitive measurement, which does not exist to this date in any system. Using Mott polarimetry, we probed the spin degrees of freedom and demonstrated that topological quantum numbers are completely determined from spin texture–imaging measurements. Applying this method to Sb and Bi1–xSbx, we identified the origin of its topological order and unusual chiral properties. These results taken together constitute the first observation of surface electrons collectively carrying a topological quantum Berry's phase and definite spin chirality, which are the key electronic properties component for realizing topological quantum computing bits with intrinsic spin Hall–like topological phenomena.
Co-reporter:D. Hsieh,
D. Qian,
L. Wray,
Y. Xia,
Y. S. Hor,
R. J. Cava
&
M. Z. Hasan
Nature 2008 452(7190) pp:970
Publication Date(Web):2008-04-24
DOI:10.1038/nature06843
When electrons are subject to a large external magnetic field, the conventional charge quantum Hall effect1, 2 dictates that an electronic excitation gap is generated in the sample bulk, but metallic conduction is permitted at the boundary. Recent theoretical models suggest that certain bulk insulators with large spin–orbit interactions may also naturally support conducting topological boundary states in the quantum limit3, 4, 5, which opens up the possibility for studying unusual quantum Hall-like phenomena in zero external magnetic fields6. Bulk Bi1-xSbx single crystals are predicted to be prime candidates7, 8 for one such unusual Hall phase of matter known as the topological insulator9, 10, 11. The hallmark of a topological insulator is the existence of metallic surface states that are higher-dimensional analogues of the edge states that characterize a quantum spin Hall insulator3, 4, 5, 6, 7, 8, 9, 10, 11, 12, 13. In addition to its interesting boundary states, the bulk of Bi1-xSbx is predicted to exhibit three-dimensional Dirac particles14, 15, 16, 17, another topic of heightened current interest following the new findings in two-dimensional graphene18, 19, 20 and charge quantum Hall fractionalization observed in pure bismuth21. However, despite numerous transport and magnetic measurements on the Bi1-xSbx family since the 1960s17, no direct evidence of either topological Hall states or bulk Dirac particles has been found. Here, using incident-photon-energy-modulated angle-resolved photoemission spectroscopy (IPEM-ARPES), we report the direct observation of massive Dirac particles in the bulk of Bi0.9Sb0.1, locate the Kramers points at the sample’s boundary and provide a comprehensive mapping of the Dirac insulator’s gapless surface electron bands. These findings taken together suggest that the observed surface state on the boundary of the bulk insulator is a realization of the ‘topological metal’9, 10, 11. They also suggest that this material has potential application in developing next-generation quantum computing devices that may incorporate ‘light-like’ bulk carriers and spin-textured surface currents.